You can delete files from OneDrive to remove them from the cloud and any devices connected to your OneDrive account.
You can temporarily stop OneDrive from syncing in the "Help & Settings" menu of the OneDrive notification area icon.
I've been moving away from OneDrive for a while, but the latest problem I encountered is the final straw. I'm unimpressed that Microsoft encouraged me to sync my desktop to OneDrive, and that it also ...
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